Mode-locked Thulium-Doped Fiber Lasers
based on Highly Ge-doped Fibers
D. Klimentov, V. V. Dvoyrin and I. T. Sorokina
Department of Physics, Norwegian University of Science and Technology, Høgskoleringen 5, Trondheim, Norway
1 RESEARCH PROBLEM
Thulium-doped ultrashort pulsed fiber lasers (TDFs)
attract increased attention due to their broad gain
spectrum extending from 1.8 to 2.1 μm (Hanna,
1990; Barnes, 1990), possibility to produce high
power and highly efficient tunable femtosecond
pulses (Wu, 2007; Jackson, 2007; Sorokina, 2014) in
the very interesting for many practical applications
wavelength range around 2 μm (Dvoyrin, 2014;
Sorokina, 2014), including eye-safe LIDAR,
medicine, high resolution spectroscopy and remote
sensing (Sorokina, 2014).
In the wavelength region of 2 μm silica-based
fibers typically exhibit anomalous group delay
dispersion (GDD). Therefore, without dispersion
compensation TDF lasers are restricted to soliton
operation, which has been demonstrated with
different mode-locking schemes (Nelson, 1995;
Sharp, 1996; Solodyankin, 2008). Alternatively,
elements for dispersion compensation can be
implemented in the cavity, enabling the laser to
operate in the stretched-pulse regime. This regime is
characterized by breathing dynamics that reduces the
total nonlinear phase shift and allows for relatively
high pulse energies compared to the fundamental
soliton regime, while the pulses can still be
compressed to very short durations outside the
resonator (Nelson, 1997).
Anomalous dispersion regime in the simple
dispersion uncompensated fiber laser leads to the
typical limitation of both pulse energy and duration
to picojoules and picoseconds, respectively.
However, implementation of dispersion
compensation usually requires additional
components, specialty fibers, i.e., holey fibers, or
even bulk elements. This technique leads to the
complexity of the scheme and decreases its
reliability. Such specialty fibers often have fragile or
mechanical splices with conventional silica-based
fibers; the insertion of bulk elements substantially
decreases the laser performance. The Ge-doped Tm-
codoped silica-based fibers with anomalous
dispersion have already shown to be effective as a
laser material (Rudy, 2012). The possibility of high
doping of such fibers with Tm allows improving the
quantum efficiency (Rudy, 2012) and decreasing the
length of the active fiber. Highly Ge-doped silica-
based fibers exhibit normal dispersion in the 2 μm
wavelength region. Such fibers naturally allow
constructing an all-fiber laser with normal cavity
dispersion. Excellent mechanical properties and
close relation to the conventional silica-based fibers
allow good reliable solid splices of the highly
germanium-doped fibers with the conventional ones.
The final construction is simpler and allows
producing femtosecond pulses as it will be revealed
in what follows. This makes such fibers promising
for producing of particularly short, power scalable
mode-locked pulses. The first works, on producing
stable continuous-wave lasing were reported in
(Dvoyrin, 2011; Dvoyrin, 2010).
2 OUTLINE OF OBJECTIVES
In this work, we present our first results and the
perspectives of the development of the Tm-doped
fiber laser based on active fibers of normal
dispersion. We propose the first femtosecond
SESAM mode-locked all-fiber laser based on the
highly Ge-doped thulium-doped normal dispersion
active fiber. In this article we focus our attention on
three particular configurations: laser operating in the
anomalous cavity dispersion regime, laser operating
in the regime of nearly zero cavity dispersion and
laser operating in the normal cavity dispersion
regime without the use of the additional dispersion
compensating elements. The pulses were amplified
by a compact TDF MOPA laser system.
For the nearly zero and normal cavity dispersion
regimes the femtosecond pulses with several
nanojoule energy were obtained at the wavelength of
around 1.88 nm. The pulses were compressed down
to 800 fs using a simple fiber compressor
represented by a piece of a conventional fiber.
80
Klimentov D., Dvoyrin V. and Sorokina I..
Mode-locked Thulium-Doped Fiber Lasers based on Highly Ge-doped Fibers.
Copyright
c
2015 SCITEPRESS (Science and Technology Publications, Lda.)
3 STATE OF THE ART
There are several demonstrations of passively mode-
locked TDF lasers, using various mechanisms of
mode-locking. These demonstrations include
nonlinear polarization rotation (NPR) (Sharp, 1996;
Wang, 2010), semiconductor saturable absorber
mirrors (SESAM) (Sharp, 1996), carbon nanotube
based saturable absorbers (Solodyankin, 2008; Kieu,
2009) and graphene based saturable absorber
(Zhang, 2012). For instance, Nelson et al.
demonstrated NPR-based mode-locked thulium fiber
laser with 500 fs pulses generation (Nelson, 1995).
In another work, Sharp et al. used a semiconductor
SESAM in a TDF laser to achieve 190 fs pulses
(Sharp, 1996). More recently, Engelbrecht et al.
reported a laser with grating-based dispersion
compensation and double-clad TDF. The laser
operated in the stretched pulse regime (Engelbrecht,
2008) with pulse energy as high as 4.3 nJ and de-
chirped pulse duration around 300 fs. Mode-locked
operation of dispersion-compensated TDF lasers has
also been successfully demonstrated (Solodyankin,
2008; Haxsen, 2008).
4 METHODOLOGY
A mode-locked TDF laser has been built using the
all-fiber linear cavity configuration. The TDF was
produced by the modified chemical vapor deposition
method. It had 55% mol.% concentration of GeO
2
in
the core (Dvoyrin, 2011; Dvoyrin, 2010; Dvoyrin,
2011). The schematic of the laser and the amplifier
are shown in Fig.1.
The cavity was formed with a SESAM saturable
absorber, a fiber coupler used for launching pump
radiation into the cavity, a piece of 3 m length of the
TDF with a highly Ge-doped core of 3μm diameter
and NA of 0.49, a fiber loop mirror with the output
coupling of 5%, and a piece of the conventional
telecommunication fiber (SMF-28). Excellent
mechanical properties and close relation to the
conventional silica-based fibers allow good reliable
solid splices of the TDF with the conventional ones.
The measured splice loses were found to be 1.5 dB
per splice. The length of the SMF-28 fiber was
varied in order to investigate the laser performance
in the wide range of the cavity dispersion. It is worth
noting that all the components used in the fiber laser
had fiber outputs based on the SMF-28 fiber.
The amplifier was based on a piece of 14 m
length of the same TDF. The laser was pumped by
one or two laser diodes (Princeton Lightwave Inc.)
operating at the wavelength of 1550 nm and 1630
nm, depending on the configuration, while for the
pumping of the amplifier we used an Er-doped fiber
laser operating at the wavelength of 1.61 μm (IPG
Photonics Inc.)
Figure 1: The schematic of the TDF laser (red frame) and amplifier (blue frame).
Mode-lockedThulium-DopedFiberLasersbasedonHighlyGe-dopedFibers
81
5 STAGE OF THE RESEARCH
5.1 Experimental Results
5.1.1 Anomalous and Nearly Zero Cavity
Dispersion Regimes
The maximum output average power for both
anomalous dispersion configurations of the laser
oscillator was 1.9 mW with 0.7% slope efficiency.
The laser emission wavelength was centered around
1.88 μm. The dispersion of the fibers is of 35±1 and
-15±1 ps/nm*km for the SMS-28 fiber and for the
TDF, respectively, at the laser emission wavelength
(Klimentov, 2012). In our experiments the cavity
dispersion varied in the range of 0.002-0.404 ps/nm
when changing the SMF-28 fiber length from 1.35 to
12.8 m. For our particular configurations: laser
operating in the anomalous cavity dispersion regime
and laser operating in the regime of nearly zero
cavity dispersion, the cavity dispersion was
0.148±0.005 and 0.002±0.001 ps/nm, respectively.
The corresponding pulse energies inside the laser
cavity were found to be 1.6 and 3.2 nJ. These energy
values noticeably exceed the values obtained in
frames of the soliton theory, which can be estimated
as 0.11 and 2.45 nJ, but may be explained by the
stretched-pulse or “dispersion management” regime
(Tamura, 1995; Tamura, 1993), where the pulses
travel through the fiber spans of alternating
dispersion and experience stretching and
recompression in every resonator round trip. As the
average pulse duration in the resonator can be
increased, the pulse energy can be increased
accordingly.
After amplification of the pulses we achieved the
average output power of 86 mW at the repetition rate
of 12 MHz corresponding to the pulse energy of 7.3
nJ and 3.7 nJ for the longer and shorter cavity,
respectively, with the amplifier slope efficiency of
3.8%.
The spectrum and autocorrelation trace for the
cavity dispersion of 0.148±0.005 ps/nm are shown in
Fig. 2(a), indicating 1.68-ps pulses with the spectral
full width at half maximum (FWHM) of 2.7 nm. The
length of SMF-28 fiber was 5.5 m and the length of
TDF was 3 m. The time-bandwidth product was 0.43
indicating that the pulses were not transform-limited.
In that regime the laser was self-starting and the
central wavelength was 1879 nm. With the cavity
dispersion decrease the mode-locking threshold
decreased slightly (from 155 to 145 mW of the
pump power); however, the maximum output power
of the laser and the amplifier remained at the same
level as previously, while the emission spectrum was
broadened from 2.7 to 5.2 nm and the pulse duration
reduced from 1.68 ps to 900 fs.
1870 1875 1880 1885 1890
-2
0
2
4
6
8
10
12
14
16
-10-8-6-4-20246810
0,010
0,011
0,012
0,013
0,014
0,015
0,016
Inten sity
Delay, ps
pulse = 1.68 ps FWHM
a/c = 2.6 ps FWHM
Optical intensity, a.u.
Wavelength, nm
FWHM 2.7 nm
(a)
1870 1875 1880 1885 1890 1895
-4 -2 0 2 4
0,014
0,015
0,016
0,017
0,018
0,019
0,020
0,021
Inten sity, a.u.
Delay, ps
pulse = 900 fs FWHM
a/c = 1.4 ps FWHM
Optical intensity, a.u.
Wavelenght, nm
FWHM 5.2 nm
(b)
Figure 2: Spectra and autocorrelations for the mode-
locked TDF laser operating in anomalous dispersion
regime (a), and the mode-locked TDF laser with the nearly
zero cavity dispersion (b).
The spectrum and autocorrelation trace for the
nearly zero cavity dispersion of 0.002±0.001 ps/nm
are shown in Fig. 2(b), indicating 900-fs pulses with
the FWHM of 5.2 nm and the repetition rate of 23.5
MHz. In that configuration the laser produced
transform-limited pulses with the sech
2
pulse shape
and the time-bandwidth product of 0.315. For this
configuration the length of SMF-28 fiber was 1.35 m
and the length of the TDF fiber was 3 m.
The key feature of this work is the use of the
highly Ge-doped active fiber with normal dispersion
at 2 µm. Passive highly Ge-doped fibers can be used
for dispersion compensation of the conventional
silica-based fibers known to have high anomalous
dispersion in the 2 µm spectral region. Same fibers
doped with thulium can significantly reduce the
complexity of a laser scheme allowing achieving the
zero cavity dispersion or even normal dispersion
without the use of separate pieces of an active fiber
PHOTOPTICS2015-DoctoralConsortium
82
and a dispersion compensation fiber.
5.1.2 Normal Cavity Dispersion Regime
It is known that the highest pulse energies can be
obtained in the normal cavity dispersion regime. So,
we have modified the laser cavity by changing its
length thus changing the cavity dispersion from
anomalous to normal and studied the performance of
the laser.
All the SMF-28 fiber pieces were removed from the
cavity, except the short fiber ends of the couplers
and the fiber loop mirror. In this configuration the
rest of SMF-28 fiber length was 68 cm resulting in
the total cavity dispersion of -0.02±0.001 ps/nm.
The mode-locking threshold in the normal cavity
dispersion regime decreased to 90 from 145 mW.
The laser remained self-starting. The emission
central wavelength was slightly blue-shifted to 1868
nm due to change of the SESAM mirror position
during reconfiguration of the laser.
The radio frequency (RF) spectrum measured
with 200 kHz frequency span and 1 kHz resolution
Figure 3: Measured RF spectrum of mode-locked output:
with a 200 kHz frequency span and 1 kHz resolution
bandwidth (upper); with a 200 MHz frequency span and
100 kHz resolution bandwidth, showing a broad spectrum
of harmonics (lower).
bandwidth is shown in Fig. 3 (upper). The repetition
rate of the laser was 26.78 MHz. A graph at the Fig.
3 (lower) illustrates the RF spectrum recorded in the
200 MHz frequency span and 100 kHz resolution
bandwidth, showing a broad spectrum of harmonics.
No signs of dual-pulsing have been observed.
Since the intracavity pulse energy was not
limited in this regime by the fundamental soliton
energy, we increased the pump power of the laser by
adding the second pump diode. The average
maximum output power of the laser reached 2.3 mW
100 200 300 400 500 600
0,0
0,5
1,0
1,5
2,0
2,5
0,5%
Otput power, mW
Launched pump power, mW
Equation
y = a + b*x
Weight
No Weighting
Residual Sum
of Squares
0,09784
Pearson's r
0,9919
Adj. R-Square
0,98263
Value Standard Error
B
Intercept -0,05398 0,05626
B
Slope 0,00467 1,65939E-4
Figure 4: The laser slope efficiency.
0 500 1000 1500 2000
0
10
20
30
40
50
60
70
(a)
3,3%
Otput power, mW
Launched pump power, mW
Equation
y = a + b*x
Weight
No Weighting
Residual Sum
of Squares
650,64605
Pearson's r
0,97866
Adj. R-Square
0,95666
Value Standard Error
B
Intercept 5,60962 1,33345
B
Slope 0,03328 0,00113
1850 1860 1870 1880 1890
(b)
Optical intensity, a.u.
Wavelenght, nm
2.4 mW
45.5 mW
54.8 mW
58.6 mW
61.5 mW
64.5 mW
Figure 5: The amplifier slope efficiency (a) and the
evolution of the spectrum after amplification (b).
Mode-lockedThulium-DopedFiberLasersbasedonHighlyGe-dopedFibers
83
and was limited by the available pump only. The
laser slope efficiency is shown in Fig. 4.
After the amplification of the pulses with the
same amplifier we achieved the average maximum
output power of 70 mW with the repetition rate of
26.8 MHz corresponding to the pulse energy of 2.6
nJ with the amplifier slope efficiency of 3.3%. The
amplifier slope efficiency and the evolution of the
spectrum after amplifier are shown in Fig. 5. As it
can be seen, the amplification did not change the
shape of the spectrum.
The spectrum and autocorrelation trace for the
laser operating in normal dispersion regime with the
cavity dispersion of -0.02±0.001 ps/nm are shown in
Fig. 6, indicating 1.35-ps pulses with the spectral
FWHM of 9 nm.
It is worth noting that the launched pump power
exceeded the specification limit of the input coupler
of the amplifier. To avoid damage we placed it in a
water tank to allow a better heat dissipation. We
believe that the visible bending of the amplifier
efficiency curve is caused by the thermal effects
inside the coupler.
1840 1850 1860 1870 1880 1890 1900 1910
-4-3-2-101234
pulse = 1.35 ps FWHM
a/c = 2.09 ps FWHM
Intensity, a.u.
Delay, ps
FWHM 9 nm
Optical intensity, a.u.
Wavelenght, nm
Figure 6: Spectrum and autocorrelation for the mode-
locked Tm-doped laser operating in normal dispersion
regime.
5.1.3 Pulse Compression
The pulses of the TDF laser operating in normal
dispersion regime after amplification were
compressed using the fiber compressor, Fig. 1. The
compressor was formed by the SMF-28 fiber. The
optimal length of fiber for the efficient compression
was found to be 3.2 m. It was found, that elongation
of this length by several meters weakly affected the
pulse duration. The Fig. 7 shows the autocorrelations
of the mode-locked pulses before the compression,
and after the compression with two lengths of the
SMF-28 fiber of 3.2 and 8 m. With the compressor
of the optimal length the initial pulses were
compressed from 1.35 ps down to 800 fs and the
spectrum was broadened from 9 to 10 nm FWHM.
The increase of the compressor length in 3 times,
approximately, did not lead to the sufficient change
in the pulse duration; the pulses from the 8 m
compressor were only slightly longer.
-4-3-2-101234
(a)
pulse = 1.35 ps FWHM
a/c = 2.09 ps FWHM
Intensity, a.u.
Delay, ps
-3 -2 -1 0 1 2 3
(b)
pulse = 800 fs FWHM
a/c = 1.24 ps FWHM
Intensity, a.u.
Delay, ps
-3 -2 -1 0 1 2 3
(c)
pulse = 910 fs FWHM
a/c = 1.41 ps FWHM
Intensity, a.u.
Delay, ps
Figure 7: The autocorrelations of the mode-locked pulses
from the Tm fiber laser operating in normal dispersion
regime: before the compression (a), the autocorrelation
measured after the compression by 3.2 m compressor (b),
and the compression by the SMF-28 with the length 8 m
(c).
5.2 Discussion
As compared to the conventional approach, we
suggest a simpler scheme with a higher reliability.
No additional dispersion-compensation, e.g. any
PHOTOPTICS2015-DoctoralConsortium
84
fibers or bulk elements, was used in our laser.
However, it operated in the normal dispersion
regime. It is worth to note, that the operation near
zero cavity dispersion allowed us to produce
femtosecond pulses directly from the oscillator in
contrast to the picosecond laser with essential
anomalous dispersion. Variation of remaining length
of the pieces of the input/output conventional
anomalous dispersion fibers from the components
used in the laser naturally allowed us to carry out a
simple form of the dispersion management resulted,
however, in femtosecond pulse generation. The
compression of the pulse from the normal-dispersion
laser was naturally provided by the laser output
piece of the conventional fiber and allowed us to
achieve the shortest, 800 fs pulses. At the same time
the pulses energy was as high as 2.6 nJ. The whole
system exhibited a much simpler level of complexity
than the conventional fiber lasers with dispersion
compensation. This is a noticeable improvement of
the mode-locked fiber laser construction.
Excellent mechanical properties and close
relation to the conventional silica-based fibers allow
good reliable solid splices of the highly germanium-
doped fibers with the conventional ones. The
measured splice losses were found to be 1.5 dB per
splice. It is worth noting that a standard fusion
splicer program was used. The splice loss can be
reduced in future by modification of the electrical
fusion splicer program or use of fibers with similar
mode diameters.
5.3 Conclusion
We have demonstrated the first femtosecond
SESAM mode-locked TDF laser based on the active
fiber with highly Ge-doped core with the normal
dispersion in the spectral region near 2 µm. The
change of the length of the conventional
telecommunication fiber inside the laser cavity
allowed variation of the total cavity dispersion in the
range of -0.02-0.404 ps/nm. The stable laser
operation was obtained in three different dispersion
regimes: laser operating in the anomalous cavity
dispersion regime, laser operating in the regime of
nearly zero cavity dispersion, and laser operating in
the normal cavity dispersion regime. The lasers
operated at the wavelength of ~1.88 µm. The pulses
from the master oscillator were amplified in the
core-pumped TDF amplifier based on the same
active fiber as the laser.
The amplification resulted in the output power of
86 mW corresponding to the pulse energy of 7.3 and
3.7 nJ for the laser cavity dispersion of 0.148 and
0.002 ps/nm, respectively. In the case corresponding
to the nearly zero cavity dispersion, the laser
produced transform-limited soliton pulses with the
time-bandwidth product of 0.315 and the pulse
duration of 900 fs, with the spectral FWHM of 5.2
nm.
For the laser operating in the normal cavity
dispersion regime the amplification resulted in the
output power of 70 mW corresponding to the pulse
energy of 2.6 nJ. The laser produced pulses with the
pulse duration of 1.35 ps, with the FWHM of 9 nm.
Finally, we could compress the pulses down to
800 fs by using the all-fiber compressor, based on
the SMF-28 fiber.
6 EXPECTED OUTCOME
The laser output power is limited by the available
pump power only; we predict, based on our
calculations, that further optimization resulting in
the efficiency increase will allow us to demonstrate
more than an order of magnitude higher pulse
energies, as there is no fundamental limitations for
the pulse energy in the normal-dispersion laser
except for the thermal load and the material damage
threshold.
Evidently, all the regimes can be improved by
the reducing of the splice losses, by the use of the
highly Ge-doped active fibers with higher
concentration of Tm, and, for the normal dispersion
cavity regime, by applying higher pump power,
which is planned for the near future experiments.
Nevertheless, the present results already demonstrate
the high potential of such fibers for producing of
ultra-short femtosecond nanojoule pulses in the
vicinity of 2 µm directly from a SESAM mode-
locked fiber oscillator.
The work was supported by the NFR projects
FRITEK/191614 and MARTEC project MLR.
The expected outcome of my research is the
reliable stable ultra-short pulsed all-fiber MOPA
system operating in the 2 μm wavelength region, as
well as the power scaling of this MOPA up to 10 W
output power by adding the second fiber amplifier
stage; design and demonstration of a fiber based
supercontinuum source and tests of the developed
laser sources for practical applications, e.g.
medicine, high resolution spectroscopy and remote
sensing.
Mode-lockedThulium-DopedFiberLasersbasedonHighlyGe-dopedFibers
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